I know the pinhole size does have a lot to do with sharpness. While a lens in focus will make an infinitely small point of light on the film, the pinhole projects a series of pinhole sized dots on the surface. Since there is no optics, there can me no reduction or enlargement.
I just did a calculation and the pinhole on the Titan is actually on the small side. For the 72mm cone, the calculations say it would need to be 0.378mm wide. But they went for a 0.35mm wide hole instead, something that would have been adequate for a 61mm cone (the smaller the cone, the smaller the hole). That's probably a big part of how sharp it really looks.